I know this list has been done to death everywhere, but I might as well throw my own thoughts out on this as well. I'll provide my reasons for my opinion as well, as some of the positions may be controversial.
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Metallica - Ride the Lightning|
Metallica - Master of Puppets|
Metallica - Kill 'Em All|
Metallica - ...And Justice For All|
Metallica - Metallica|